I remember it clearly. I've let the controller drop in frustration many times but only once have I actually -thrown- it. I was playing Illusion of Gaia, I think this fishing part. I've never been this p***ed at a game before, and that's saying something. It was funny, too, because it was very deliberate, I remember thinking "I'm going to throw this controller, I'm gonna be very careful though because I don't want anything breaking". So I got close to the screen, mentally I went "F**** YOU" and then just kinda flinged it against it. I was worried immediately because it made a nice "clink" sound, but luckily nothing broke.
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At least we got beat by a SuperNiceDog, 2011 Rivals Guru Champ!